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This collection documents the care and management of Mount Vernon through the work of the MVLA. Types of material include correspondence, reports, memos, notes, personal and biographical information, news clippings, meeting agendas, photographs, scrapbooks, and ephemera. Several highlights of the collection include the original minutes of Council meetings, scrapbooks and ledgers created by Vice Regents, and early correspondence with Regents and Vice Regents. While the library's collection "Early Records of the MVLA" documents the founding and early years of the organization, the Papers of the MVLA continues where that collection ended and preserves the ongoing story of these women and the fulfillment of their mission. Creators of the collection are largely the board members themselves, along with staff and employees who worked directly with them. Scope notes have been added before the content list of each series to better describe its specific provenance and content. The bulk of the collection dates from the 1950s to the 1990s, however there is a very wide range represented overall, 1858-2016.

Professional and personal papers of Parke Shepherd Rouse, Jr. who was a newspaper writer and columnist and an author of books on Virginia.

Papers, 1933-1978, of Ted Dalton, Virginia state senator, 1944-1959; Republican candidate for governor of Virginia in 1953 and 1957; and U.S. District judge for the Western district of Virginia. Includes correspondence, speeches, news clippings, photographs, recordings, reels of film and legal opinions.

The University Archives Audiovisual Collection is an artificial collection of various audio and visual formats documenting the College of William and Mary campus, events, people, etc. The collection contains analog, magnetic, and digital media and while not comprehensive, it does include material from a variety of time periods and types of events including commencements, Charter Day, building dedications, lecture series, Raft Debates, visiting scholars and distinguished guests, athletic events, and much more. Researchers are encouraged to verify with staff the format of individual items and availability for immediate use. Many items in the collection will require preservation reformatting before they can be used.