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This collection holds the historic financial records of the MVLA including accounting ledgers, tax documents, insurance papers, receipts, invoices, payroll lists, annual and quarterly budgets, financial statements and reports, policies, contracts, correspondence, and other miscellaneous items. Records in this collection contain information on the Association's financial accounting, revenue, expenditures, employees and employee benefits, investments, taxes, and other financial concerns. There is a very limited amount pertaining to fundraising efforts and/or private donations, which can be found in the files of Mount Vernon's development department (currently unprocessed). Bulk date 1870s-2000s.

The University Archives Audiovisual Collection is an artificial collection of various audio and visual formats documenting the College of William and Mary campus, events, people, etc. The collection contains analog, magnetic, and digital media and while not comprehensive, it does include material from a variety of time periods and types of events including commencements, Charter Day, building dedications, lecture series, Raft Debates, visiting scholars and distinguished guests, athletic events, and much more. Researchers are encouraged to verify with staff the format of individual items and availability for immediate use. Many items in the collection will require preservation reformatting before they can be used.

This collection contains the entirety of General Samuel Vaughan Wilson's personal and professional papers, as donated to Hampden-Sydney College by his widow in 2019. Topics include the Vietnam and Second World Wars, the development of the United States of America's intelligence and counter-intelligence communities, military strategy, and Wilson's role as president of Hampden-Sydney College from 1992 until 2000.

The Edward Watson Hook papers reflect his wide-ranging professional activities related to heading the Department of Internal Medicine, participating in the larger Health System/University processes, and pursuing his own research and external activities. The documents detail Hook's direct personal participation in professional organizations and also show the wide range of details he coordinated in running the department of internal medicine. A noteworthy aspect of the collection includes an unpublished History of the Department of Medicine written by Byrd Leavell. Hook read and critiqued the manuscript, but Leavell died before completing the book. Also, Hook conducted a series of interviews with Thomas H. Hunter which complement with the Thomas H. Hunter papers, MS-4, Claude Moore Health Sciences Library.

Inventoried collection of correspondence, poems, essays, mementos, and personal effects of Elizabeth Carrington Eggleston, daughter of former Hampden-Sydney College President Joseph DuPuy Eggleston, including numerous "jotting books" or commonplace books that Eggleston kept throughout her life.