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This collection holds the historic financial records of the MVLA including accounting ledgers, tax documents, insurance papers, receipts, invoices, payroll lists, annual and quarterly budgets, financial statements and reports, policies, contracts, correspondence, and other miscellaneous items. Records in this collection contain information on the Association's financial accounting, revenue, expenditures, employees and employee benefits, investments, taxes, and other financial concerns. There is a very limited amount pertaining to fundraising efforts and/or private donations, which can be found in the files of Mount Vernon's development department (currently unprocessed). Bulk date 1870s-2000s.

Summary article on adoption of ICC Statute by Committee of the Whole of the Rome Conference

These are the collected papers of Alexandria politician Armistead Lloyd Boothe (1907-1990). Papers created or collected by Boothe in the course of his career include campaign materials, correspondence with colleagues, and extensive newspaper clippings in addition to other research on political issues such as segregation, education, and transportation.

This collection consists of ca. 3,000 items, (13 Hollingers and 15 oversize bound volumes), ca. 9 linear shelf feet), ca. 1907-1949, chiefly the genealogical correspondence and research of William D. Ligon, Jr.concerning the Ligon family. The collection contains correspondence, newsclippings, photographs, post cards, photostats, forms, genealogical charts, book reviews, Christmas card albums, and printed material, much of it mounted in bound volumes and scrapbooks. Also present is the typescript and illustrations for the book The Ligon Family and Connections,the product of all of the research and genealogical inquiries conducted by Ligon through his correspondence.

Papers of Russell L. Davisson, a Republican member of the West Virginia State House of Delegates. Includes mostly genealogy records regarding the Davison, Davisson, and Davidson Families; also includes political correspondence with Governor Arch Moore (1967-1972) and material regarding the welfare system in Mingo County (1966-1967).

Series III of the William Faulkner Collection contains the personal papers, files, belongings, and related realia of William Faulkner. Materials in the collection range in date from 1824 to 2003 and are divided into eight subseries: William Faulkner's working papers related to his literary works, drawings made by Faulkner, his childhood ephemera and student records, military and flight records, family papers, honors and awards, belongings and related realia, and reminiscences or accounts of William Faulkner.

The Historical Photograph Collection is largely comprised of materials created by or for the Mount Vernon Ladies' Association. Some of the earliest photographs of the estate were created and sold to visitors by the Association as a means of income. Those efforts helped to establish an important collection of 19th century views. The collection spans the 1850s to 2000s and includes over 140 linear feet of analog material providing a visual history of the Mansion, outbuildings, tombs, grounds, events, visitors, collection objects, personnel, and changes throughout the estate.