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The Historical Photograph Collection is largely comprised of materials created by or for the Mount Vernon Ladies' Association. Some of the earliest photographs of the estate were created and sold to visitors by the Association as a means of income. Those efforts helped to establish an important collection of 19th century views. The collection spans the 1850s to 2000s and includes over 140 linear feet of analog material providing a visual history of the Mansion, outbuildings, tombs, grounds, events, visitors, collection objects, personnel, and changes throughout the estate.

This collection, consisting of ca. 760 items, (5 Hollinger boxes, 22-1/2 linear shelf inches), includes the papers of the Woods Familyof Albemarle County, Virginia, from 1847 to 1926. Correspondence comprises the major part of the collection and deals with a variety of subjects. The correspondence between Micajah Woodsand his parents during the Civil War includes detailed descriptions of the campaigns and battles in which he fought, among them the battles of Port Republic, Second Manassas, Crampton's Gap, Sharpsburg, New Market, Second Cold Harbor, Lynchburg, Fisher's Hill, and Monocacy. The men under whom he served included "Stonewall" Jackson, J. E. B. Stuart, and John Floyd. A portion of the post-Civil War correspondence regards Civil War Veterans' Reunions and recollections of battles and campaigns.

(includes signature of Washington Irving

The Low Moor Iron Company papers consist of approximately 280 four-inch Hollinger archives boxes (ca. 95 linear feet) of records, ca. 1885-1927, and some 1200 bound volumes of the company's accounting records, 1873-1927, of this iron producing company located in Low Moor (four miles southwest of Clifton Forge), Alleghany County, Virginia.

Papers of Ellen Anderson Gholson Glasgow include drafts of and notes on several novels including Phases of an inferior planet,Vein of iron,A certain measure,In this our life, and The woman within, as well as copies of speeches and articles, and notes relating to her personal and literary affairs.

This collection holds the historic financial records of the MVLA including accounting ledgers, tax documents, insurance papers, receipts, invoices, payroll lists, annual and quarterly budgets, financial statements and reports, policies, contracts, correspondence, and other miscellaneous items. Records in this collection contain information on the Association's financial accounting, revenue, expenditures, employees and employee benefits, investments, taxes, and other financial concerns. There is a very limited amount pertaining to fundraising efforts and/or private donations, which can be found in the files of Mount Vernon's development department (currently unprocessed). Bulk date 1870s-2000s.