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Series 1: Group A, Acc. 78 T97 and 1992.63: Papers, 1856-1895, of John Tyler, Jr., post Civil War Republican Party activist. Subjects covered by the collection include alcoholism, Republican Party politics, Presidential elections, political patronage, Reconstruction, Methodist Episcopal Church, Florida, Braxton Bragg, and the Fenian Brotherhood. Prominent correspondents include Charles Francis Adams, Chester Alan Arthur, Pierre G. T. Beauregard, James Gillespie Blaine, James Buchanan, Jefferson Davis, Benjamin Stoddert Ewell, Henry Stuart Foote, Nathan Bedford Forrest, James A. Garfield, John Brown Gordon, Horace Greeley, Wade Hampton, Rutherford B. Hayes, Andrew Johnson, Joseph Eggleston Johnston, L. Q. C. Lamar, William Mahone, Raphael Semmes, William Henry Seward, John Sherman, Leroy Pope Walker, and William Lowndes Young. Acc. 1992.63 consists of letters of John Tyler, Jr., son of the President, to Mrs. Laura Holloway, author of a book on the ladies of the White House. Letters written from Washington, D.C.

This collection includes materials from Dr. Emory L. Kemp's career of researching, documenting, and preserving historic structures. Kemp was a practicing civil engineer from 1952-1959, then taught civil engineering, historic preservation, and the history of technology from 1962-2003 at West Virginia University. He served as an expert consultant for the preservation of many historic engineering structures, including bridges, waterways, and mills. He also published regularly and remained active in several professional organizations.

This record group contains papers and projects created by students as part of their coursework, such as honors theses and capstone papers.

Papers of Ellen Anderson Gholson Glasgow include drafts of and notes on several novels including Phases of an inferior planet,Vein of iron,A certain measure,In this our life, and The woman within, as well as copies of speeches and articles, and notes relating to her personal and literary affairs.

The Historical Photograph Collection is largely comprised of materials created by or for the Mount Vernon Ladies' Association. Some of the earliest photographs of the estate were created and sold to visitors by the Association as a means of income. Those efforts helped to establish an important collection of 19th century views. The collection spans the 1850s to 2000s and includes over 140 linear feet of analog material providing a visual history of the Mansion, outbuildings, tombs, grounds, events, visitors, collection objects, personnel, and changes throughout the estate.

Family papers compiled by Katherine Williams of Berkeley Springs, West Virginia. Most of the papers are of the James H. Taylor family of Clarksburg, West Virginia dating from the 19th century. There are also records of the Irwin family including a genealogy, and the Civil War letters of private George Irwin, a soldier in Company F, 95th Ohio Volunteer Infantry. Other families documented include the Redman and Summers families. The collection includes letters, autograph books, family business records, genealogies, photographs, and other material.