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The records of the Alumni Association of the College of William and Mary include office files, material from select Executive Secretaries, meeting minutes, publications, correspondence, and other material documenting the activities of the William & Mary Alumni Association as well as the College of William & Mary's history and alumni more generally.

Personal and professional papers of Amos Ralph Koontz, surgeon. The personal papers, 1865-1986, include the correspondence of Koontz, his wife, Besse (Stocking) Koontz and their son, James William Koontz. Included are travel diaries, documents concerning the College of William and Mary and Johns Hopkins and material relating to social clubs and societies. The professional papers contain correspondence relating to Koontz' medical practice, political material, documents pertaining to military service, memberships in professional organizations, and newspaper and magazine article reprints.

The collection contains letters and programs, writings and other papers documenting Aquilla Matthews, an African-American woman originally from Danville, Virginia who was the director of the USO African American Women's group, The Sun and Sand Caravan during World War II. The collection includes: photographs of several members of the group notes with description of different areas served and several letters documenting Matthews personal and professional life.

The bulk consists of reel-to-reel tapes and cassettes created by the Public Relations Office (now Communications and Marketing) which recorded VMI events. Also includes Glee Club LPs (1950's-60's) and misc. other audio (e.g. Flapjack Blues played by Frank Pancake).

The Berlin B. Chapman Papers consists of postcards, photographs, books, and manuscript materials documenting Chapman's personal life and professional career. The bulk of the collection pertains to materials related to education, including Chapman's own academic experiences as well as the history of educational institutions and the teaching profession in Marion County and central West Virginia.

This collection contains correspondence, other documents, and photographs pertaining to Dr. Beverley Randolph Tucker, his son Beverley Randolph Tucker II, and their families, most prominently being Elizabeth Sloan Tucker Cann, wife of Beverley Randolph Tucker II.

Collection of letters and documents of the Braun and Jung families from the 19th and 20th centuries. The earliest documents are a prenuptial agreement, dowry agreement, and will from the middle 1800's (photocopies). The documents are in German, but an English translation accompanies most items. The collection includes a "Familien Stammbuch" or family genealogy book along with two ancestry passports for Gunter Braun and Ernst Jung. They were used to prove familial background in Nazi Germany.

The personal and professional papers of Carter Lowance, executive assistant to six governors of Virginia: William M. Tuck, John S. Battle, Thomas B. Stanley, J. Lindsay Almond, Albertis S. Harrison and Mills Edwin Godwin. Papers also concern Harry F. Byrd, Sr. and Harry F. Byrd, Jr., and John N. Dalton. There are speeches, papers relating to Lowance's military career (including correspondence with his wife, Elizabeth Austin Lowance), awards received by Lowance, photographs, and papers concerning his funeral. There is also correspondence received by Mrs. Lowance after his death. The collections includes material concerning proposed amendments to the Virginia Constitution as well as some papers concerning Lowance's service with the College of William and Mary.