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The Historical Photograph Collection is largely comprised of materials created by or for the Mount Vernon Ladies' Association. Some of the earliest photographs of the estate were created and sold to visitors by the Association as a means of income. Those efforts helped to establish an important collection of 19th century views. The collection spans the 1850s to 2000s and includes over 140 linear feet of analog material providing a visual history of the Mansion, outbuildings, tombs, grounds, events, visitors, collection objects, personnel, and changes throughout the estate.

Views of Mount Vernon spanning more than 100 years. The Robert Waldsmith Collection consists of approximately 300 stereographs and cabinet cards by Alexander Gardner, N. G. Johnson, Luke D. Dillon, and others. Highlights of the collection include: several west front views of the Mansion, including the earlist known one by Frederick Langenheim, circa 1856; an early view of the tomb, circa 1857, and a collection of Washington statues and buildings honoring the first President.

Collection contains 14 albumen photographs, most stamped "Bena F. Harrison," five captioned in pencil. Some images depict locations in Loudon County, including James Monroe's Oak Hill, the Point of Rocks Bridge, and another unidentified home. Other Virginia mansions are depicted, including the "Lutz House. No. Va." Some images depict a church in Petersburg.

Artificial collection of photographs obtained from various sources. Please see container inventory for more information.

Letters, a speech, and a photograph relating to the abolitionist movement in the United States. Correspondents include: Theodore Dwight Weld (1803-1895) of Lane Seminary, Elizur Wright (1804-1885), Secretary of the American Anti-Slavery Society, Gerrit Smith (1797-1874), philanthropist and reformer, Henry Grew (1782-1862), Quaker abolitionist, William Lloyd Garrison (1805-1879), prominent abolitionist, and Parker Pillsbury (1809-1898), abolitionist author. Subjects include abolition tactics and organizations, expressions of sympathy to Garrison on the death of his wife and publication of Pillsbury's work. Also includes a photograph of Mary Grew (1813-1896), daughter of Henry Grew and an abolitionist in her own right.

A collection of 27 8x10 silver gelatin prints that includes photographs of Dana Abraham's family. Each photograph is black and white with white borders, and spans from Fall 2022 to Spring 2023. Most of the photographs are of young women and girls of the Abraham family, with some elderly members of the family also included. The photographs are representative of the Abraham family's bond. Statement from creator and donor Dana Abraham: "The bond my family shares is something truly extraordinary. I wanted to capture special moments with my family to provide them with a means of documenting our shared love and experiences. Some of the works focus on my sisters and the tribulations of youth, while others expand the rest of the family, portraying the intimate nature of familial bonds"

Letters of Pvt. Adam Porter of Company A, 194th Pennsylvania Infantry Regiment, stationed at Camp Carroll, Md. to his sister and brother-in-law in Williamsport, Pa. He describes camp life. Included is a pen and ink sketch of Porter and a carte-de-visite of him in uniform.