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The collection includes: correspondence and land records of Robert "King" Carter; correspondence and land records of his sons Robert Carter (1704-1731) and Landon Carter (1710-1778); correspondence, accounts, land records and the appointment to the Virginia Council of Robert Carter (1728-1804), son of Robert Carter (1704-1731); correspondence, diaries, land records and accounts of Robert Wormeley Carter (1734-1804), son of Landon Carter of Sabine Hall; and correspondence and land records and papers concerning the estate of Robert Carter's grandson, Landon Carter (1757-1820).

This collection covers the history of the Cazenove Family of Alexandria from the 1790s to the 1970s. The first part of the collection features records from James O'Hara Cazenove (1880-1971), consisting primarily of correspondence and records relating to his business interests and investments, as well as legal documents and business related litigation. Some of the correspondence and notebooks relate to his role as an inventor including a patent for an improved eggbeater from the 1920s. It also includes records from his brother, Louis A. deCazenove (1851-1925), primarily related to his education at Cornell University.

Letters, accounts, and legal papers of Dr. Charles Brown. Collection includes letters, 1813-1818, concerning patients (including slaves).

The Charles Campbell papers consist of papers received or collected by Charles Campbell (1807-1876), Virginia historian. The papers fall into four general headings: historical papers collected by Charles Campbell, correspondence, manuscript volumes, and miscellaneous. These include personal and professional correspondence as well as eighteenth century documents collected by Charles Campbell, newspaper clippings, diaries, scrapbooks, and notebooks, covering then period 1743-1896. The papers reflect Charles Campbell's interests in history, teaching, newspaper editing, railroad engineering, politics, genealogy, publication of his works, and the town of Petersburg where he lived for most of his life.

The collection includes the correspondence, certificates, photographs, accounts, and journals of Rear Admiral Charles H. Bell. Naval journals cover Bell's service in the Mediterranean Sea from 1855-1858. The photographs are a mix of personal and souvenirs, which largely depict men and women from Peru. There is also material related to his role as executor for the estate of Samuel Swartwout. The collection also includes papers related to the Smith family, particularly Bell's executor and son-in-law, Israel Smith, Jr. Of particular note is a broadside of Thomas Jefferson's first inaugural address (given on March 4, 1801) printed on silk by W. Pechin Print.

Papers, 1826-1872, of Charles Dimmock and Charles Henry Dimmock. Includes sketch of the life of Charles H. Dimmock; a manuscript volume containing a journal of a voyage from Norfolk to Madeira and farm journal of "Shabby Hall," Gloucester County, Va.; travel diary, 1826, of Charles Dimmock concerning travels in Venice and Germany; and papers concerning the service of Charles Henry Dimmock in the engineer's corps in the Confederate Army, some of which include work at Yorktown, Va. and having enslaved individuals build ramparts at Petersburg, Va.

Letters received by John Philip Cline, a Lutheran clergyman at New Market, Va and Smithburg, Washington County, Md. Includes fourteen letters, 1824-1832, written by John G. Morris concerning his education; the Henkel family; his pastorate; and [Samuel Simon] Schmucker.

The collection also contains miscellaneous manuscripts and account books. Included in this material are: land grants, 1761 and 1766, for land in Fairfax and Frederick counties, Va.; eighty-five survey maps of Frederick, Fauquier, and Loudoun counties, Va. and Berkeley and Hampshire counties, W. Va.; road petitions, 1743-1828, for Frederick County; affidavits for Revolutionary War service; correspondence, 1923-1930, of the Improved Order of Redmen, Great Council of Virginia; letters written to W. H. H. Flick; account books of merchants in Frederick County, , Lexington, Va. and Harrisonburg, Va.; and account books of the Richmond Whig (1837), the Lexington Gazette; and the Southern Collegian (student newspaper at Washington and Lee College). There is also a daybook which contains copies of letters, notes and bonds written by Philip Nelson to Powhatan R. Page; notes on the Washington and Custis families and the building of "Arlington"; and notes concerning John Randolph of Roanoke and the Underwood Constitutional Convention in Richmond.

Letters, chiefly 1919-1964, written by Mary Haldane Begg Coleman (1875-1967) of Williamsburg, Virginia, to Julia Gardiner Tyler Wilson (1881-1965), of Charlottesville, Virginia. Diaries of Mary Haldane Begg Coleman and Isabella Haldane.