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There are 84 items, 1716-1865, chiefly letters of Angelica Schuyler Church(1756-1815) and other family members, including her husband John Barker Church, brother-in-law Alexander Hamilton(1757-1804), father Philip John Schuyler, and brother-in-law Stephen van Rensselaer(1764-1839). Other notable correspondents include: Justus Erich Bollman(1769-1821); Charles James Fox(1749-1806); Thomas Jefferson(1743-1826); Marquis de Lafayette(1757-1834); Abraham Lincoln(1809-1865); Winfield Scott(1786-1866); Baron von Steuben(1730-1794); Charles Maurice de Talleyrand-Perigord(1754-1838); and, George Washington(1732-1799).

The collection primarily contains correspondence of the Randolph family and Nicholas family. Several land title records are also present.

The Bushrod Washington Family Papers consist of documents gathered by the descendants of the first President of the United States, George Washington. The collection comprises an assortment of correspondence and legal documents documenting the lives and property ownership of several branches of the Washington family. The collection is organized into five series: Correspondence, Legal Documents, Social, Miscellaneous, and Indenture Notices (Land Deeds).

This collection consists of the papers of the Randolph Family of Edgehill, (commonly called the Edgehill-Randolph Papers) and the Wilson Cary Nicholas papers, ca. 787 items (6 Hollinger boxes, 2.5 linear shelf feet), ca. 1765-1869, and undated.

This collection contains high-resolution digital images of rare legal texts. The Arthur J. Morris Law Library created these images for its "1828 Catalogue Project."

This collection consists of papers inherited and collected by Washington family descendants. Many were purchased in 1927 at auction to reunite Washington family correspondence. The collection includes correspondence, financial documents and legal documents that relate primarily to the Custis and Lewis families, but include other items related to Virginia history. Charles and Peter Chapin, the previous owners of this collection, descended from Eleanor Parke Custis and Lawrence Lewis through Esther Maria Lewis and Charles Chapin. This collection was originally assembled by Esther Maria Lewis Chapin who inherited some of the Washington/Custis papers, but was also an avid collector and brought back together family items that were being dispersed nationwide. This collection is an example of that effort; much of which was at auction in 1927 (Anderson Galleries, sale 2201, 28-29 November 1927).

The collection comprises mostly of anatomical illustrations of humans and animals by professional medical illustrators and medical practioners, but there is a good number of caricatures. Many of the images depict 20th century surgical prodedures; there are also physiological illustrations included in the collection. Most items are drawn in pencil on illustration paper with cardboard backing. In addition, there are some drawings in notepads and on tracing paper.

The collection contains 41 manuscripts dating 1770-1831. Many of the manuscripts date from the era of the American Revolution, and several are directly relevant to the course of the war. Among the documents are single letters by John Adams, Aaron Burr, Benjamin Franklin, Alexander Hamilton, John Hancock, Patrick Henry, John Jay, Thomas Jefferson, Lafayette, James Madison, John Marshall, James Monroe, Paul Revere, and George Washington, as well as letters and other documents that include the signatures of signers of the Declaration of Independence.

This collection consists of letters written by and addressed to Thomas Jefferson, as well as architectural plans and studies that were created or endorsed by Jefferson, created by other individuals associated with him, deeds, plats, and maps, some of which pertain to the subjects of the architectural studies, and other miscellaneous materials.