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The bulk of this collection is made up of letters from Jane Charlotte Washington to her son, John Augustine Washington III. Also included are letters to Eleanor Love Selden Washington, a few letters to or from John Augustine Washington III to various individuals, several letters from George Mason of Hollin Hall (1797-1870) to John Augustine Washington III, letters by Lackland and Alexander family members (relatives of the Washingtons) and three receipts. The subject matter of most letters is family or personal affairs and Mount Vernon business with some discussion of the enslaved people owned by the Washingtons. Inclusive dates are 1837 to 1861.

The collection contains correspondence between John Augustine Washington III and his wife Eleanor Love Selden. The letters begin during the Washingtons' engagement and continues through eighteen years of marriage, ending with a letter from John Augustine to Eleanor composed the day prior to her sudden death. The letters contain information on family matters, the management of the Mount Vernon estate, and plantation life prior to the Civil War.

This collection concerns the inheritance, maintenance, and sale of the Mount Vernon estate by its last private owner, John Augustine Washington III. A large majority of the collection is correspondence to or from John Augustine Washington III with a significant portion relating to the purchase of the estate by the Mount Vernon Ladies' Association. Three diaries kept by John Augustine are also included and contain important information about his slaves, agricultural practices, and finances. Other types of material in the collection include legal documents, receipts, photographs, and ephemera. Photocopies were made for most of the manuscripts and can be viewed as surrogates to the originals.

This collection includes correspondence between John Augustine Washington III and his mother and wife, as well as other family members, mostly dealing with family matters and running Mount Vernon.