- "George Washington" Miniseries Collection, 1981/19861
- Anniversaries and Commemorations Collection, 1981/20001
- Audio Visual Collection, 1928/20151
- Beebe collection of Washington family papers, 1818/1861, bulk 1840/18501
- Bushrod Washington family papers, 1662/18351
- Chapin collection of Washington & Custis family documents, 1758/18291
- Early Records of the Mount Vernon Ladies' Association, 1853/1951, bulk 1853/18751
- Edith Sprouse Subject Files, 1960/19861
- Elizabeth Bordley Gibson collection, 1794/18511
- Emma Read Ball Genealogical Research Files, 1911/19121
- Esther Maria Lewis Chapin collection of Washington family documents, 1743/18521
- Financial Records of the Mount Vernon Ladies' Association, 1858/20151
- Frances Abbott Lyon Papers, 1976/19831
- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/20171
- George Washington Memorial Parkway History Collection, 1900/20011