- 1907 Jamestown Exposition, St. Paul's Episcopal Church Records, 1907/19081
- A. Rufus Tonelson Papers, 1922/19751
- A.E.S. Stephens Papers, 1949/19611
- Admiral John Randolph Tucker Papers, 1865/18971
- Albert I. Godden Papers, 1949/19721
- Albert S. Armentrout Collection, 1965/20091
- Alexander Brooks "A.B." Jackson Papers, 1965/19811
- Alice Rice Jaffe Papers, 1807/1950, bulk 1919/19501
- Allan Blank Papers, 1958/20091
- Allan G. Donn Papers, 1961/19701
- Allen-Johnson Family Papers, 1838/19471
- Allison Kenneth Scribner Papers, 1946/19761
- American Association of University Professors (AAUP) Records, 1960/19831
- American Association of University Women, Norfolk Branch (AAUW) Records, 1902/20001
- American Society of Mechanical Engineers Scrapbook, 1986/19871