- A. H. Hand Papers, 1835/20091
- Adam Empie Papers, 1811/2004, bulk 1811/18501
- Alpha Delta Gamma Records, 1993/20123
- Alpha Phi Alpha Kappa Pi chapter records, 1972/20114
- Alumni Association Photograph Collection, 1960/2010, bulk 1970/19902
- Alumni Association Records, 1833/2014, bulk 1950/200554
- Alumni Band Organization Records, 1986/2012, bulk 1986/20007
- American Studies Program Records, 1960/20061
- Ann Buckles Papers, 1950/200873
- Ann Marie Stock Cuban Poster collection, 1967/20151
- Anne H. Cutler Papers, 1930/2013, bulk 1954/20008
- Archibald F. Ward, Jr. Papers, 1939/2007, bulk 1945/19601
- Armand J. Galfo Papers, 1940/2008, bulk 1958/19954
- Art Song of Williamsburg Records, 2000/200711
- Association for the Preservation of Virginia Antiquities, Yorktown Branch Records, 1921/2013, bulk 1975/20051