- Robert E. Marshak Papers, 1933/1995356
- Rick Boucher Papers, 1968/2017, bulk 1975/2011303
- John T. Parsons Papers, 1910/2000281
- Arthur M. Squires Papers, 1888/1987, bulk 1940/1987169
- Records of the Virginia Cooperative Extension, 1862/1997148
- Dr. Richard Zallen Papers, 1940/2007130
- W. Dale Parker Papers, 1914/200695
- Records of the Office of the President, William E. Lavery, 1975/198793
- Roanoke Appalachian Trail Club Records, 202593
- George Green Shackelford Papers, 1899/1990, bulk 1955/198983
- William Hewitt Phillips Papers, 1918/200881
- The Road Company Records, 1972/199879
- James I. Robertson Jr. Papers, 1849/201178
- Sigrid L. Rupp Architectural Collection, 1950/200472
- Alfred C. Payne Collection, 1917/200363