- Albert L. Sturm Papers, 1904/1988109
- Albert S. Armentrout Collection, 1965/20091
- Alberta Pfeiffer Architectural Collection, 1929/19762
- Alexander Brooks "A.B." Jackson Papers, 1965/198151
- Alexander G. Gilliam collection of University of Virginia history papers, 1921/20194
- Alexander Mahood, Architect, Drawings for West Virginia University Building Projects, 1955/19794
- Alexander Theroux letters to Judy Barnes, 1973/19801
- Alexandria Antique Arts Association Collection (MS134), 1971/19999
- Alexandria Bicentennial Commission (MS085), 1937/19792
- Alexandria Black Family Reunion Digital Collection, 1937/20058
- Alexandria Gazette I (MS331), 1942/19961
- Alexandria History Collection (MS240), 1767/200820
- Alexandria Hospital School of Nursing records, 1894/19871
- Alexandria Library Board Records (MS416), 1937/20208
- Alexandria Library Company Records (MS002), 1794/200720