- Papers of the Mount Vernon Ladies' Association, 1858/2016150
- Restoration Files for the Historic Structures Report, 1750/2005141
- Papers of the Superintendent and Resident Director, 1850/1996137
- Mount Vernon Black and White Film Collection, 1933/200537
- Financial Records of the Mount Vernon Ladies' Association, 1858/201532
- Operation Overview Collection, 1953/198331
- Papers of Christine Meadows, Curator, 1960/199730
- Publications Committee Collection, 1951/199723
- Publications and Printed Material of the Mount Vernon Ladies' Association, 1854/201614
- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/201712
- Historic ephemera collection, 1796/198610
- Historical Photograph Collection, 1850/201010
- Publications - History of Mount Vernon and George Washington, 1854/20127
- Audio Visual Collection, 1928/20156
- Edith Sprouse Subject Files, 1960/19865