- Adolphus DeBussey, Soldier, Civil War Letters1
- Aerial Photographs of the Virginia Dept. of Transportation,1
- African American GI's Vietnam and West Germany Scrapbook1
- African American Hugh Carr family, River View Farm, and the Papers of the Ivy Creek Foundation1
- African American programs and photographs from Roanoke, and Wytheville, Virginia1
- Agnes Smith (1906-1994), Author, Correspondence, Manuscripts, and Publications1
- Agnes Smith (1906-1994), Author, Literary Manuscripts1
- Agnes Smith (1906-1994), Author, Papers1
- Agricultural Extension Service Records1
- Al Gross Papers1
- Alan Clarke Railroad Research Papers1
- Albemarle County Medical Society records1
- Albert E. Garrett, Jr. scrapbook1
- Albert E. Haak Scrapbook1
- Albert I. Godden Papers1