- Administration records collection, 1776/19761
- Alumni and VMI certificates and citations collection, 1860/20132
- Fitzgerald Flournoy papers, 1912/19631
- Fortnightly Club Papers, 1900/20151
- Frank J. Gilliam Papers, 1914/19641
- Frank Parsons papers, 1891/19991
- Frederick William McWane papers, 1909/1959, bulk 1909/19131
- Freeman Hansford Hart Collection, 1910/19651
- Historical Photograph Collection, 1850/20101
- James Bernard Merrick Collection, 1927/1970, bulk 1927/19301
- James Graham Leyburn collection, 1902/19932
- John Grier Varner Papers, 1905/1978, bulk 1926/19781
- Leslie Cheek, Jr. Personal Papers (SC-02), 1931/19931
- Letitia Pate Evans Papers, 1947/19921
- Lexington, Virginia, 1818/19911