- Allison Kenneth Scribner Papers, 1946/19763
- Alpha Sigma Alpha Collection, 1933/20188
- Alpha Tau Chapter of Kappa Alpha Psi minute books (Bluefield State University, West Virginia), 1951/19641
- Althea Hunt Papers, 1926/196118
- Alton D. Brashear papers, 1935/19551
- Alumni Association Photograph Collection, 1960/2010, bulk 1970/19901
- Alumni Association Records, 1833/2014, bulk 1950/200558
- Alumni Association Records, 1924/201615
- Alumni Association Records, 1950/20075
- Alumni and VMI certificates and citations collection, 1860/20132
- Alumni biographical files - University of Virginia School of Law, 1901/19971
- Alvena V. Seckar, Author and Artist, Artwork and Papers, 1940/19681
- Alvena V. Seckar, Author and Artist, Manuscripts and Correspondence, 1940/19681
- Alvena V. Seckar, Author and Artist, Writings, Photographs, Scrapbooks, and Other Material, 1927/20056
- Alvin Duke Chandler Papers, 1896/1984, bulk 1950/196021