- Alice Constance Burford Booth Papers, 1940/19684
- Alice Huffman Bugel Collection (Eighth Evacuation Unit Hospital), 1942/20001
- Alice Langley Hsieh Papers, 1943/19783
- Alice McMechen, Collector, Papers of Artist Alvena V. Seckar, 1945/20082
- Alice Rice Jaffe Papers, 1807/1950, bulk 1919/19505
- Aline Jeannette (Vier) Shrum Papers, 1946/19581
- Allan T. Gwathmey collection, 1914/19491
- Allard Hostetter Diaries, 1925/19491
- Alleghany Chapter, National Society of the Daughters of the American Revolution Records, 1890/202219
- Allen-Kean-Laurence family letters, 1837/19602
- Alliance of Women in Architecture (AWA) Records, 1992/19981
- Allison Kenneth Scribner Papers, 1946/19763
- Alpha Sigma Alpha Collection, 1933/20187
- Althea Hunt Papers, 1926/196122
- Alton D. Brashear papers, 1935/19551