- Alexandria Hospital School of Nursing records, 1894/19871
- Alexandria Library Board Records (MS416), 1937/20203
- Alexandria Library Company Records (MS002), 1794/200711
- Alexandria Library Records (MS098), 1937/20139
- Alexandria National Bank Collection (MS193), 1904/19781
- Alexandria Office of Sheriff Jail Records (MS054), 1891/19484
- Alexandria, Virginia City Records (MS019), 1750/1983, bulk 1825/18751
- Alfred A. Bolton, Papers regarding History of Management and Other Material, 1900/200733
- Alfred C. Payne Collection, 1917/200332
- Alfred Dickinson Barksdale Papers
1905-197314
- Alfred P. Upshur collection, 1909/19531
- Alfred R. Armstrong Papers, 1928/19761
- Alfred W. Lawson Collection, 1913/19483
- Alice Cartledge Cornett, Journalist, Papers, 1945/2017, bulk 1973/19921
- Alice Combs Scrapbook, 1946/19481