- Alleghany Chapter, National Society of the Daughters of the American Revolution Records, 1890/202215
- Allen Caperton Braxton Papers2
- Allen Family Papers, 1766/19337
- Allen and Margaret Cook Collection, 1900/19431
- Allen-Johnson Family Papers, 1838/19473
- Allen-Kean-Laurence family letters, 1837/19602
- Alston Gordon Dayton Papers, 1846/19392
- Althea Hunt Papers, 1926/196121
- Alumni Association Records, 1833/2014, bulk 1950/200527
- Alumni Association Records, 1924/20165
- Alumni Association Records, 1950/20072
- Alumni and VMI certificates and citations collection, 1860/20132
- Alumni biographical files - University of Virginia School of Law, 1901/19971
- Alvena V. Seckar, Author and Artist, Writings, Photographs, Scrapbooks, and Other Material, 1927/20053
- Alvin D. Chandler Naval Record, 1925/19511