- A. E. Dick Howard papers, 1928/20171
- A. J. Gustin Priest papers, 1919/19761
- Addison H. Smith papers, 1917/1970, bulk 1917/19221
- African American Hugh Carr family, River View Farm, and the Papers of the Ivy Creek Foundation, 1916/19881
- African-American owned Virginia businesses letters and ephemera, 1919/19331
- Albert Frederick Wilson papers, 1840/19341
- Alderman family papers, 1779/19611
- Alexander G. Gilliam collection of University of Virginia history papers, 1921/20191
- Alexander Wylie Moore miscellaneous papers, 1896/19501
- Alexandria Hospital School of Nursing records, 1894/19871
- Alicia Wertenbaker Flynn letters, 1930/19441
- Alumni Day records, 1900/19791
- Alumni biographical files - University of Virginia School of Law, 1901/19971
- American Lung Association of Virginia (ALAV) collection, 1907/20041
- American Rhododendron Society Records, 1927/20221