- Alfred C. Payne Collection, 1917/20034
- Alfred Dickinson Barksdale Papers
1893-194016
- Alfred Dickinson Barksdale Papers
1905-19736
- Alfred P. Upshur collection, 1909/19531
- Alfred W. Lawson Collection, 1913/19481
- Algernon B. Chandler, Jr. Records, 1912/192811
- Alice Maud Jones and Burton Family Pins, 1890/19291
- Alice Rice Jaffe Papers, 1807/1950, bulk 1919/19503
- Alice Virginia Kellam Scrapbook, 1923/19252
- Allan T. Gwathmey collection, 1914/19491
- Allard Hostetter Diaries, 1925/19491
- Alleghany Chapter, National Society of the Daughters of the American Revolution Records, 1890/202211
- Allen Caperton Braxton Papers2
- Allen Family Papers, 1766/193311
- Allen and Margaret Cook Collection, 1900/19431