- Alumni and VMI certificates and citations collection, 1860/20131
- Barton family papers, 1855/18691
- Board of Visitors correspondence and administrative records, historical, 1846/19371
- Cadet Life, Organizations, and Activities, 18451
- Commandant of Cadets Historical Records, 1839/19501
- Department of Physics Miscellaneous Historical Records, 1906/19501
- Financial and business records, historical, 1839/19642
- Historical Grade Books, 1840/19191
- Jennings C. Wise papers, 1910/19601
- Leonard T. Gerow papers, 1911/19701
- Matriculation Books, 1839/19941
- Moses J. Ezekiel papers, 1867/19171
- Nathaniel C. Wilson collection, 1834/19411
- New Market collection, 1894/19151
- Office of the Superintendent correspondence, 1840/19182