- Early Records of the Mount Vernon Ladies' Association, 1853/1951, bulk 1853/18751
- Financial Records of the Mount Vernon Ladies' Association, 1858/20157
- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/20171
- George Washington Memorial Parkway History Collection, 1900/20011
- Harrison H. Dodge Papers, 1816/19364
- Historic ephemera collection, 1796/19862
- Land Records of the MVLA, 1858/20061
- Papers of Christine Meadows, Curator, 1960/19973
- Papers of the Mount Vernon Ladies' Association, 1858/201645
- Papers of the Superintendent and Resident Director, 1850/199653
- Peter family papers, 1722/19322
- Publications and Printed Material of the Mount Vernon Ladies' Association, 1854/20167
- Restoration Files for the Historic Structures Report, 1750/2005146
- Taylor collection of Lewis family papers, 1700/19501