- A.S. Hammack papers, 1864/19541
- Account Books, 1782/18951
- Ackerly Family Papers4
- Adele Goodman Clark papers, 1849/19783
- Alexander Brown Papers (I), 1815/19104
- Alexandria Black Family Reunion Digital Collection, 1937/20051
- Alfred C. Garnett, Jr. Papers
1868-19454
- Alfred Dickinson Barksdale Papers
1893-19401
- Alfred Dickinson Barksdale Papers
1905-19731
- Alfred Spates Papers
1843-19092
- Alice Barber Stephens Collection
1892-19073
- Allen Caperton Braxton Papers3
- Allen-Kean-Laurence family letters, 1837/19601
- Alumni and VMI certificates and citations collection, 1860/20131
- Andrew Monroe Cridler Papers, 1871-1913, n.d.1