- Inge Horton Architectural Collection, 1964/199953
- Thomas Browse Family Papers, 1785/1942, bulk 1830/191052
- Virginia Counties Collection, 1600/2000, bulk 1730/189052
- Richard Wright collection, 1806/201749
- Snyder Family papers, 1850/190149
- Sheet Music Collection, 1827/197448
- Ancella Bickley, Historian, Research Papers regarding African-Americans, 1775/2018, bulk 1970/201145
- Ellison A. Smyth, Jr. Papers, 1859/192745
- Jim Comstock, Newspaper Editor and Collector, Papers, 1650/2003, bulk 1850/199545
- Austin-Twyman Papers, 1765/193944
- Oren F. Morton (1857-1926) Papers, 1799/192643
- Bell, Kent, Cloyd, Withrow Family Collection, 1780/199841
- W.E. Bibb Papers
1830-194040
- James Washington Singleton Papers, 1770/1975, bulk 1850/192039
- Papers of the Mount Vernon Ladies' Association, 1858/201639