- Bushrod Washington family papers, 1662/18353
- Chapin collection of Washington & Custis family documents, 1758/18291
- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/20171
- George Washington collection, 1654/179923
- Historic ephemera collection, 1796/19861
- Historic manuscript collection, 1601/193339
- Historic map collection, 1675/19711
- Historic newspapers collection, 1757/19577
- Lawrence Lewis family papers, 1785/18582
- Martha Washington collection, 1761/18024
- Peter family papers, 1722/19324
- Restoration Files for the Historic Structures Report, 1750/20051
- Richard H. Brown Revolutionary War Map Collection, 1740/17991
- Taylor collection of Lewis family papers, 1700/19501
- Ted and Mary Wendell early American collection, 1721/18261