- Records of Superintendent Francis H. Smith, 1839-1889, 1839/188912
- Archibald M. Fauntleroy papers, 18572
- Charles A. Derby papers, 1839/18912
- Charles P. Deyerle papers, 1842/18552
- Office of the Superintendent correspondence, 1840/19182
- William D. Stuart papers, 1850/18632
- Barton family papers, 1855/18691
- Board of Visitors correspondence and administrative records, historical, 1846/19371
- Carl M. Best papers, 1884/18861
- Charles R. K. Varner collection, 1881/19111
- F. H. Smith Letter, 18671
- Francis H. Smith Circular Letter Soliciting Items to Establish a Museum at VMI, 18451
- George A. Goodman papers, 1848/18651
- Henry Edmundson Letters, 1814/18471
- James H. Waddell papers, 1855/18791