- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/20179
- Andrew C. L. Gatewood papers, 1860/19932
- Historic ephemera collection, 1796/19862
- Title:: Rev. Samuel Huntting Sayre, Jr. Papers 1874-19891920-19602
- Virginia Cities Collection, 1663/19802
- A. Edwin Kendrew Papers, 1930/19591
- Agnes Mason Price papers, 1930/19351
- Archibald F. Ward, Jr. Papers, 1939/2007, bulk 1945/19601
- Armand J. Galfo Papers, 1940/2008, bulk 1958/19951
- Arthur Franklin Raper papers, 1959/19751
- Ash Lawn-Highland records, 1978/19981
- Audie Scott Tilghman papers, 1925/19301
- Auxiliary Services records, 1962/20191
- Aviation Brochures and Pamphlets Collection, 1910/19581
- Bird and Bull Press Collection1