- College of Education History Records, 1970/19901
- College of Education Restructuring Records, 1979/19961
- Dan H. Pletta Papers, 1942/19961
- Dean Carter Papers, 1950/2003, bulk 1964/19821
- Doris Zallen Papers, 1952/20161
- Dorothy McCombs Collection,, 1970/19891
- Dr. Richard Zallen Papers, 1940/20071
- Earl A. Thornton Papers, 1885/20001
- Edgemont Farm Papers, 1925/19981
- Elizabeth D. Guthrie Papers on the VPI Glee Club, 1940/19881
- Felix Sebba Papers, 1979/19891
- Frank J. Maher Papers, 1934/19861
- G. Burke Johnston Papers, 1900/19931
- G. Preston Frazer Collection, 1939/20031
- George Collins Papers, 1952/19931