- A. H. Hand Papers, 1835/20091
- Agnes Wolf papers, 1966/20061
- Alpha Delta Gamma Records, 1993/20121
- Alumni Association Records, 1833/2014, bulk 1950/20051
- Alumni Band Organization Records, 1986/2012, bulk 1986/20001
- American Studies Program Records, 1960/20061
- Ann Buckles Papers, 1950/20081
- Archibald F. Ward, Jr. Papers, 1939/2007, bulk 1945/19601
- Armand J. Galfo Papers, 1940/2008, bulk 1958/19951
- Art Song of Williamsburg Records, 2000/20071
- Association for the Preservation of Virginia Antiquities, Yorktown Branch Records, 1921/2013, bulk 1975/20051
- Blacksburg Baptist Church Records, 1894/20071
- Board of Visitors records, 1757/20231
- Bryant Mangum American literature collection, 1920/20221
- C-SPAN records, 1809/2012, bulk 1978/20121