- Alfred R. Armstrong Papers, 1928/19761
- Alumni Association Records, 1833/2014, bulk 1950/20051
- Alvin Duke Chandler Papers, 1896/1984, bulk 1950/19601
- Ann Zimmerman Kulp Scrapbooks, 1951/19561
- Autograph Album (Williamsburg, Va.), 1925/19581
- Beverly Simonton Kelly Letters, 1949/19981
- Board of Visitors records, 1757/20231
- Calendars Collection, 1910/20131
- Carl R. Dolmetsch Papers, 1751/19901
- Carlton Casey Papers, 1894/19991
- Carter Lowance Papers, 1860/1993, bulk 1942/19881
- Catherine Dennis Papers, 1918/1974, bulk 1918/19211
- Cecil McCulley Papers, 1945/2005, bulk 1945/19771
- Channing Moore Hall Papers, 1920/1953, bulk 1930/19531
- Charles J. Duke, Jr. Papers, 1919/19581