- James Towne Collony Pottery Papers, 1937/1962, bulk 1937/19401
- John L. Tunstall papers, 1866/18671
- Kenneth W. Newman Records, 1971/20042
- Li Jen Sun collection, 1940/19451
- Martha Washington collection, 1761/18021
- Mount Vernon Black and White Film Collection, 1933/20052
- Newton D. Baker Letter to Otto Miller, 19361
- Pace Family Papers, 1947/20061
- Pompeo Cecchetti book of poems, 18951
- Print Collection, 1740/19401
- Scottish Coalition USA Archives, 1980/20111
- Thomas E. Pugh Papers, 1914/2001, bulk 1941/19981
- Virginia G. Gray Cookery Collection, 1830/19701
- Woodbridge Family Papers, 1927/20011